It does sound that there are more than a couple of issues with the set up the pump possibly being 1 of the.
You could look at separating the floors out and fitting an individual pump to each circuit, less work for each pump and if one fails still got the other 3 floors going!
You say you keep adding apartments and rads, every time you added a rad did you take the flow and returns back to the primaries of from the nearest feeds?
Are all the rads in the system re-balanced when you add a new one?
The rads are 600 x 1000 are they sized for the room at -20 you want bigger than standard I would think, our calcs work on about -5 I think.
Is the underfloor ran from the same boiler as the 55 rads? rads pulling 100ish KW how much does the underfloor pull all from a 66kw boiler?
Just a couple of thoughts for you to mull over!